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    Por favor, use este identificador para citar o enlazar este ítem:https://uvadoc.uva.es/handle/10324/75066

    Título
    Superchiral light emerging from bound states in the continuum in metasurfaces of Si nanorod dimers
    Autor
    Pura Ruiz, José LuisAutoridad UVA
    Castillo López de Larrinzar, Beatriz
    Liang, Minpeng
    García Martín, Antonio
    Gómez Rivas, Jaime
    Sánchez Gil, José A.
    Año del Documento
    2024
    Editorial
    ACS (American Chemical Society)
    Descripción
    Producción Científica
    Documento Fuente
    ACS Photonics, 2024, vol. 11, n. 10, p. 4090-4100
    Abstract
    Bound states in the continuum (BICs) in all-dielectric metasurfaces enhance light–matter interaction at the nanoscale due to their infinite Q factors and strong field confinement. Among a variety of phenomena already reported, their impact on chiral light has recently attracted great interest. Here we investigate the emergence of intrinsic and extrinsic optical chirality associated with the excitation of BICs in various metasurfaces made of Si nanorod dimers on a quartz substrate, comparing three cases: parallel nanorods (neutral) and shifted and slanted dimers, with/without index-matching superstrate. We analyze both the circular dichroism (CD) of the far-field (FF) interaction and the helicity of the near-field (NF) distribution. We show that the best approach to achieve chiral response in the FF based on extrinsic chirality is to exploit quasi-BICs (q-BICs) appearing in the case of slanted nanorod dimers. By contrast, the helicity density is largely enhanced in the case of shifted dimers, as it presents intrinsic chirality, with values 2 orders of magnitude larger than those of circularly polarized plane waves. These so-called superchiral electromagnetic fields concentrated at the nanoscale within the metasurface hold promise of appealing implications in phenomena such as strong-coupling, photoluminescence emission, or other local light–matter interactions.
    Materias Unesco
    22 Física
    Palabras Clave
    Superchiral light
    Bound states in the continuum
    Chirality
    Helicity
    Near-field
    ISSN
    2330-4022
    Revisión por pares
    SI
    DOI
    10.1021/acsphotonics.4c00938
    Patrocinador
    Ministerio de Ciencia e Innovación (TED2021-131417B-I00, PID2022-137569NB-C41, PID2021-126046OB-C22 and PID2020-113533RB-C33)
    Ministerio para la Transición Ecológica y el Reto Demográfico/FEDER (TED2021-130786B-I00)
    Unión Europea (101098813)
    Unión Europea-NextGenerationEU y Ministerio de Ciencia e Innovación (PRTR-C17.I1)
    Unión Europea-Margarita Salas (CONVREC-2021-23)
    Version del Editor
    https://pubs.acs.org/doi/10.1021/acsphotonics.4c00938
    Propietario de los Derechos
    © 2024 The Authors
    Idioma
    eng
    URI
    https://uvadoc.uva.es/handle/10324/75066
    Tipo de versión
    info:eu-repo/semantics/publishedVersion
    Derechos
    openAccess
    Collections
    • DEP32 - Artículos de revista [284]
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