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    Por favor, use este identificador para citar o enlazar este ítem:https://uvadoc.uva.es/handle/10324/65519

    Título
    Long-life aqueous organic redox flow batteries enabled by amidoxime-functionalized ion-selective polymer membranes
    Autor
    Ye, Chunchun
    Tan, Rui
    Wang, Anqi
    Chen, Jie
    Comesaña Gandara, BibianaAutoridad UVA Orcid
    Breakwell, Charlotte
    Alvarez Fernandez, Alberto
    Fan, Zhiyu
    Weng, Jiaqi
    Bezzu, C. Grazia
    Guldin, Stefan
    Brandon, Nigel P.
    Kucernak, Anthony R.
    Jelfs, Kim E.
    McKeown, Neil B.
    Song, Qilei
    Año del Documento
    2022
    Editorial
    Wiley
    Descripción
    Producción Científica
    Documento Fuente
    Angewandte Chemie International Edition, 2022, Volume 61, Issue 38, e202207580
    Résumé
    Redox flow batteries (RFBs) based on aqueous organic electrolytes are a promising technology for safe and cost-effective large-scale electrical energy storage. Membrane separators are a key component in RFBs, allowing fast conduction of charge-carrier ions but minimizing the cross-over of redox-active species. Here, we report the molecular engineering of amidoxime-functionalized Polymers of Intrinsic Microporosity (AO-PIMs) by tuning their polymer chain topology and pore architecture to optimize membrane ion transport functions. AO-PIM membranes are integrated with three emerging aqueous organic flow battery chemistries, and the synergetic integration of ion-selective membranes with molecular engineered organic molecules in neutral-pH electrolytes leads to significantly enhanced cycling stability.
    ISSN
    1433-7851
    Revisión por pares
    SI
    DOI
    10.1002/ANIE.202207580
    Patrocinador
    European Research Council (ERC) under the European Union's Horizon 2020 research and innovation programme (grant agreement No 851272, ERC-StG-PE8-NanoMMES) and (grant agreement No 758370, CoMMaD)
    Engineering and Physical Sciences Research Council (EPSRC, UK, EP/V047078/1)
    EPSRC Centre for Advanced Materials for Integrated Energy Systems (CAM-IES, EP/P007767/1)
    Energy SuperStore (UK Energy Storage Research Hub)
    Department of the Defense Threat Reduction Agency grant number HDTRA1-18-1-0054
    Version del Editor
    https://onlinelibrary.wiley.com/doi/10.1002/anie.202207580
    Idioma
    eng
    URI
    https://uvadoc.uva.es/handle/10324/65519
    Tipo de versión
    info:eu-repo/semantics/publishedVersion
    Derechos
    openAccess
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    • DEP63 - Artículos de revista [324]
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    Angew Chem Int Ed - 2022 - Ye - Long‐Life Aqueous Organic Redox Flow Batteries Enabled by Amidoxime‐Functionalized (1).pdf
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    14.37Mo
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    Attribution-NonCommercial-NoDerivatives 4.0 InternacionalExcepté là où spécifié autrement, la license de ce document est décrite en tant que Attribution-NonCommercial-NoDerivatives 4.0 Internacional

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