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    Por favor, use este identificador para citar o enlazar este ítem:https://uvadoc.uva.es/handle/10324/72890

    Título
    Metal- and covalent-organic framework mixed matrix membranes for CO2 separation: A perspective on stability and scalability
    Autor
    Shan, Meixia
    Geng, Xiumei
    Imaz, Ihnar
    Broto-Ribas, Anna
    Ortín-Rubio, Borja
    Maspoch, Daniel
    Ansaloni, Luca
    Peters, Thijs A.
    Tena Matias, AlbertoAutoridad UVA Orcid
    Boerrigter, Marcel E.
    Vermaas, David A.
    Año del Documento
    2024
    Editorial
    Elsevier
    Descripción
    Producción Científica
    Documento Fuente
    Journal of Membrane Science 691 (2024) 122258
    Resumen
    Membrane technology has attracted great industrial interest in carbon capture and separation owing to the merits of energy-efficiency, environmental friendliness and low capital investment. Conventional polymeric membranes for CO2 separation suffer from the trade-off between permeability and selectivity. Introducing porous fillers in polymers is one approach to enhance membrane separation performance. Metal-organic frameworks (MOFs), with ordered porous structure and diverse chemical functionalities, are promising fillers to prepare mixed matrix membranes (MMMs) for CO2 separation. However, the main issue of MOF based MMMs in industry is their stability and processability. This review analyses recent work on stable and scalable MOF based MMMs for CO2 separation. The typical stable MOFs, MOF-based MMMs and the scalable MOF synthesis are summarized. A large number of MOF-based MMM suffer from instability upon exposure to contaminants. For that reason, we also discuss the use of covalent organic frameworks (COFs) as an alternative to prepare MMMs for CO2 separation, considering their excellent stability and good compatibility with polymers. Finally, a brief conclusion and current challenges on obtaining scalable and stable MMMs are outlined. This review may provide some guidance for designing high performance MMMs for industrial CO2 capture and separation to help achieving carbon neutrality.
    Revisión por pares
    SI
    DOI
    10.1016/j.memsci.2023.122258
    Patrocinador
    European Union's Horizon 2020 - GENESIS project- Grant Agreement No. 760899
    National Natural Science Foundation of China (Nos. 52003250)
    Catalan AGAUR (project 2017 SGR 238)
    CERCA Program/Generalitat de Cata lunya. ICN2 is supported by the Severo Ochoa program from the Spanish MINECO (grant SEV-2017-0706)
    Version del Editor
    https://www.sciencedirect.com/science/article/pii/S0376738823009146
    Idioma
    eng
    URI
    https://uvadoc.uva.es/handle/10324/72890
    Tipo de versión
    info:eu-repo/semantics/publishedVersion
    Derechos
    openAccess
    Aparece en las colecciones
    • DEP31 - Artículos de revista [167]
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    JMS 2024.pdf
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    Attribution-NonCommercial-NoDerivatives 4.0 InternacionalLa licencia del ítem se describe como Attribution-NonCommercial-NoDerivatives 4.0 Internacional

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